I will use 91+, as it is false economy to do otherwise. But whereas I buy gas on the various local military bases (we got'em all, selling NAVgas, ARgas, CORPSgas, AIRgas, GUARDgas), and none of it is "Top Tier," I will be using an anti-fouling additive as noted in the N.A. smart Owners Manual (pg. 307). I'm not sure yet what the official smart recommended list is, but I have heard that M-B recommends "Techron," as used in Chevron/Texaco top tier fuels. Shell's top tier additive is "V-Power" and blended in their premium gas (only). Conoco/Phillips/76 uses "PROclean," but I don't know if it is available separately as Techron and V-Power are. There are likely others from non-gas companies.
Top Tier Gasoline